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Accounts of Chemical Research
Scopus
ISSN 0001-4842 · American Chemical Society · 29 artikel di indeks
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Alkaline Water Electrolysis for Green Hydrogen Production
High Resolution Image Download MS PowerPoint Slide Conspectus The global energy landscape is undergoing significant change. Hydrogen is seen as the energy carrier of the future and will be a key element in the development of more sustainable industry and society. However, hydrogen is currently…
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Layered Oxide Cathodes for Sodium-Ion Batteries: Storage Mechanism, Electrochemistry, and Techno-economics
High Resolution Image Download MS PowerPoint Slide Conspectus Lithium-ion batteries (LIBs) are ubiquitous in all modern portable electronic devices such as mobile phones and laptops as well as for powering hybrid electric vehicles and other large-scale devices. Sodium-ion batteries (NIBs), which…
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Electrochemical Approaches for CO2 Conversion to Chemicals: A Journey toward Practical Applications
Conspectus Carbon capture, utilization, and sequestration play an essential role to address CO 2 emissions. Among all carbon utilization technologies, CO 2 electroreduction has gained immense interest due to its potential for directly converting CO 2 to a variety of valuable commodity chemicals…
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Electrolyte Effects on CO 2 Electrochemical Reduction to CO
High Resolution Image Download MS PowerPoint Slide Conspectus The electrochemical reduction of CO 2 (CO2RR) constitutes an alternative to fossil fuel-based technologies for the production of fuels and commodity chemicals. Yet the application of CO2RR electrolyzers is hampered by low energy and…
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Reticular Chemistry for Highly Porous Metal–Organic Frameworks: The Chemistry and Applications
Conspectus Current global crises related to clean energy and the environment entail the development of materials that are capable of addressing these challenges. Metal–organic frameworks (MOFs), a class of functional materials assembled from metal-containing nodes and organic ligands via…
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Atropisomerism in the Pharmaceutically Relevant Realm
> 4.5 years). In general, class-3 atropisomers are considered to be suitable for drug development. There are currently four FDA-approved drugs that exist as stable atropisomers, and many others are in clinical trials or have recently appeared in the drug discovery literature. Class-1 atropisomers…
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Carboxylic Acids as Adaptive Functional Groups in Metallaphotoredox Catalysis
)-rich scaffolds into pharmaceutically active molecules as a means to achieve improved solubility and physiological stability, providing the impetus to develop new coupling strategies to access these challenging motifs in the most straightforward way possible. As an alternative to classical…
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Autonomous Chemical Experiments: Challenges and Perspectives on Establishing a Self-Driving Lab
We must accelerate the pace at which we make technological advancements to address climate change and disease risks worldwide. This swifter pace of discovery requires faster research and development cycles enabled by better integration between hypothesis generation, design, experimentation, and…
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Photobiocatalysis for Abiological Transformations
Harnessing biocatalysts for novel abiological transformations is a longstanding goal of synthetic chemistry. Combining the merits of biocatalysis and photocatalysis allows for selective transformations fueled by visible light and offers many advantages including new reactivity, high…
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CO 2 Reduction Using Water as an Electron Donor over Heterogeneous Photocatalysts Aiming at Artificial Photosynthesis
reduction under visible light irradiation. Moreover, introducing a conducting polymer as a hole transporter and surface modification with Ag and ZnS improve photoelectrochemical performance.
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Fluorescent Probes for Lipid Membranes: From the Cell Surface to Organelles
Conspectus Biomembranes are ubiquitous lipid structures that delimit the cell surface and organelles and operate as platforms for a multitude of biomolecular processes. The development of chemical tools─fluorescent probes─for the sensing and imaging of biomembranes is a rapidly growing research…
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Innovative Approaches to Li-Argyrodite Solid Electrolytes for All-Solid-State Lithium Batteries
Conspectus As the world transitions away from fossil energy to green and renewable energy, electrochemical energy storage increasingly becomes a vital component of the mix to conduct this transition. The central goal in developing next-generation batteries is to maximize the gravimetric and…
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Data-Driven Strategies for Accelerated Materials Design
The ongoing revolution of the natural sciences by the advent of machine learning and artificial intelligence sparked significant interest in the material science community in recent years. The intrinsically high dimensionality of the space of realizable materials makes traditional approaches…
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Navigating the Unnatural Reaction Space: Directed Evolution of Heme Proteins for Selective Carbene and Nitrene Transfer
Conspectus Despite the astonishing diversity of naturally occurring biocatalytic processes, enzymes do not catalyze many of the transformations favored by synthetic chemists. Either nature does not care about the specific products, or if she does, she has adopted a different synthetic strategy. In…
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Transition Metal (Ni, Cu, Pd)-Catalyzed Alkene Dicarbofunctionalization Reactions
Conspectus Recently, alkene dicarbofunctionalization, i.e., the powerful organic synthesis method of alkene difunctionalization with two carbon sources, emerged as a formidable reaction with immense promise to synthesize complex molecules expeditiously from simple chemicals. This reaction is…
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The RaPID Platform for the Discovery of Pseudo-Natural Macrocyclic Peptides
pseudo-natural products.
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Lipid Nanoparticle–mRNA Formulations for Therapeutic Applications
Conspectus After decades of extensive fundamental studies and clinical trials, lipid nanoparticles (LNPs) have demonstrated effective mRNA delivery such as the Moderna and Pfizer-BioNTech vaccines fighting against COVID-19. Moreover, researchers and clinicians have been investigating mRNA…
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Synthetic and Mechanistic Implications of Chlorine Photoelimination in Nickel/Photoredox C(sp 3 )–H Cross-Coupling
Conspectus In recent years, the development of light-driven reactions has contributed numerous advances in synthetic organic chemistry. A particularly active research area combines photoredox catalysis with nickel catalysis to accomplish otherwise inaccessible cross-coupling reactions. In these…
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Mechanisms of Nickel-Catalyzed Coupling Reactions and Applications in Alkene Functionalization
Conspectus Nickel complexes exhibit distinct properties from other group 10 metals, including a small nuclear radius, high paring energy, low electronegativity, and low redox potentials. These properties enable Ni catalysts to accommodate and stabilize paramagnetic intermediates, access radical…
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Polyphenol-Mediated Assembly for Particle Engineering
Conspectus Polyphenols are naturally occurring compounds that are ubiquitous in plants and display a spectrum of physical, chemical, and biological properties. For example, they are antioxidants, have therapeutic properties, absorb UV radiation, and complex with metal ions. Additionally…